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A range of dialkyl derivatives are isolated and the molecular structures of a selection are solved. The generation of the nascent species [Cr(NAr)(_2)(=CHCMe(_3))] is investigated and the conversion of Cr(NAr)(_2)(CH(_2)CMe(_3))(_2) (24) to Cr(NAr)( 2)(CHDCMe(_3))(C(_6)D(_5)) (25) is the subject of a kinetic study. In chapter 5, the ROMP of a series of amino acid derived norbomene monomers is studied.

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